Hi,
If you've already performed the Disk Cleanup procedure to clean the windows.old folder from Q&A, after the procedure you can access the folder and delete it.
Remember, if you've done the procedure, it's not possible to revert to the previous version of Windows 10.
https://apps.microsoft.com/detail/xp9m26rsclnt88?hl=pt-BR&gl=TW
A good option to check your files would be to download TreeSize, which is free, to analyze your C drive and see the large folders and files you're not using.
Remember, don't delete anything without being sure. If you use TreeSize, if you have any doubts, let me know here and I can help you.
If drives D and C are on the same SSD or HDD, you could take free space from D and put it on C to increase the available space, and I can instruct you on how to do that.
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Thanks