Apologies in delayed response.
As you have an existing LB, you need to create an inbound NAT pool configuration for a load balancer use Add-AzureRmLoadBalancerInboundNatPoolConfig cmdlet and then configure the LB with the nat pool and update the LB. After this you can set the LB.
Please check the details in this stackoverflow thread.
Also, you can look at this thread for details on Adding Inbound nat pool to existing scale set and this.
Hope this helps.
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