
Hi @Cleveland & Co
You said that "They can still open the documents, but any changes they make aren't synced back to the SharePoint library", this means these files have been downloaded to the users' PC, they are not online anymore so the changes will not be synced to SharePoint.
You could use On-Demand function to see whether the files could be seen after the user permission has been removed.
OneDrive Files On-Demand helps you access all your files in OneDrive without having to download all of them and use storage space on your device. When you turn on Files On-Demand, you’ll see all your files in Mac Finder and get new information about each file. New files created online or on another device appear as online-only files, which don’t take up space on your device. When you’re connected to the internet, you’ll be able to use online-only files like every other file on your device.
If the answer is helpful, please click "Accept Answer" and kindly upvote it. If you have extra questions about this answer, please click "Comment".
Note: Please follow the steps in our documentation to enable e-mail notifications if you want to receive the related email notification for this thread.