Try it like this:
net use r: \\nasserver\images\ TheAdminAccountsPassword /user:admin /persistent:yes
Don't use an elevated command prompt. It won't be visible in the Windows explorer unless you add a registry entry to enable that.
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Windows 10 Pro 21H2 in workgroup
Trying to access share on NAS (buffalo) in same subnet
cmd line elevated
net use r: \nasserver\images\ /user:nasserver\admin /persistent:yes
System error 67 has occurred.
The network name cannot be found.
net use * \nasserver\images /user:nasserver /persistent:yes
System error 58 has occurred.
The specified server cannot perform the requested operation.
Try it like this:
net use r: \\nasserver\images\ TheAdminAccountsPassword /user:admin /persistent:yes
Don't use an elevated command prompt. It won't be visible in the Windows explorer unless you add a registry entry to enable that.