Hi @James Frederick
Please check whether you can login this account into OneDrive online.
If you can access OneDrive online successfully, it's recommended to reset OneDrive to have a check.
In addintion, if reseting OneDrive does not work, please unlink the OneDrive account, uninstall it and reinstall it to check this issue.
- As you have synced your Mac to your personal Microsoft account, please unlink this account.
- Open the Applications folder, drag the blue OneDrive cloud to the trash, and then enter your Mac credentials.
If there is still OneDrive folder shown in Finder, I would suggest you back its files and subfolders, then try to delete it. - And then, restart your PC, I would suggest you install it again. (Please Note: Since the link is not hosted by Microsoft, the link may changed without notice. Microsoft does not guarantee the accuracy of this information.)
- Sign into OneDrive.
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