Hi @Jon E,
According to your description, Outlook works fine by removing the calendar from the Outlook profile. As soon as they connect to that SharePoint calendar, Outlook crashes.
Other SharePoint Calendars have no problem connecting to Outlook, this looks like a calendar sync issue.
Does the SharePoint calendar have many recurring events? Did the user make a change to the calendar in Outlook and it failed to sync on SharePoint?
In view of this, you may need to re-create this SP calendar in the SharePoint site to connect to Outlook to get out of the current predicament.
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