You can submit a billing support request here.
https://azure.microsoft.com/en-us/support/options/
--please don't forget to Accept as answer if the reply is helpful--
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Hi, I am getting this error while trying to register my new credit card with Azure for one year free account.
"You're not eligible for an Azure free account"
I have used an existing email ID for this new credit card unintentionally. And now I am stuck. Please let me know what I can do here. Is there any support team who I can talk to?..Please suggest.
You can submit a billing support request here.
https://azure.microsoft.com/en-us/support/options/
--please don't forget to Accept as answer if the reply is helpful--