Why do you wish to do so?
You have more than enough memory.
Shared memory is dynamically allocated.
It's worth noting that shared GPU memory is dynamically allocated by the system as needed.
If the GPU does not require it, .... it releases this behind the scenes if some other application requires it.
It doesn't permanently take away from your system memory.
It's there to supplement your dedicated GPU memory if required, but if other applications need that memory, it should be released for them to use.
Meaning that what is shared with the GPU will be released if some other applications require it.
Your computer takes care of this behind the scenes.
Cheers.