Hi Julia,
CSRSS.exe is a core system process that can't be terminated. There are two different ways to find the offending process (or service) that has locked the Ctrl key.
Option 1: Perform a clean boot. Basically, you disable all third-party programs or services via MSCONFIG. Pls see this Microsoft article for more information.
Option 2: Close all running programs. Run a Process Monitor trace and reproduce the issue by pressing Ctrl+Z a number of times until the above error window appears. After the error message appears, stop the trace and save "All events", zip the PML trace log file, upload it to OneDrive/Dropbox/WeTransfer.com and share the link here.