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In order to debug the fulltrust process in your UWP project, you will have to start the UWP process without debugging (or detach the debugger from it). Then attach to the debugger to the fulltrust process and your breakpoints will be hit.
First, please deploy your app to your device. Then run your app from the Start Menu. Please remember to start the desktop bridge app instead of a single UWP app or a single WPF app. After, go back to Visual Studio, find the Debug button on the top bar. Click the Debug and choose Attach to Process. It will show a window and you could choose the WPF process. Then you could debug the WPF app as usual.
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