Hello Randall C. Wade,
Based on your description, you cannot add a specific guest to your Office 365 group. In this scenario, please check the below two options to add external users in O365 group.
Option 1: invite people to join your group :
You can invite people to join your group. If it's a private group, the group owner will receive a request from the invitee to join the group. You can also invite guests to join the group. They'll receive group conversations and calendar events in their inbox.
However, guests can't be group owners, view the global address list, view all information on group member contact cards, or view membership of the group.
Invite people to join your group, you can refer this article:
https://support.office.com/en-us/article/add-and-remove-group-members-in-outlook-3b650f4a-5c9b-4f94-a1bb-0cca4b1091de
Option 2: Create mail contacts from EAC and add the mail contact as a member of O365 group:
Mail contacts are mail-enabled directory service objects that contain information about people or organizations that exist outside your Exchange or Exchange Online organization. Each mail contact has an external email
address.
A. Create a mail contact : Use the EAC to create a mail contact
1. In the EAC, navigate to
Recipients > Contacts.
2. Click
New
>
Mail contact.
3. Complete the following boxes on the
New mail contact page:
· First name: Use this box to type the contact's first name.
· Initials: Use this box to type the contact's initials.
· Last name: Use this box to type the contact's last name.
· * Display name: Use this box to type a display name for the contact. This is the name that's listed in the contacts list in the EAC and in your
organization's address book. By default, this box is populated with the names you enter in the
First name, Initials, and Last name boxes. If you didn't use those boxes, you must still type a name in this box because it's required. The name can't exceed 64 characters.
· * Name: Use this box to type a name for the contact. This is the name that's listed in the directory service. Like the display name, this box
is populated by default with the names you enter in the First name,
Initials, and Last name boxes. If you didn't use those boxes, you must still type a name in this box because it's required. The name can't exceed 64 characters.
· * Alias: Use this box to type an alias (64 characters or less) for the contact. This box is required.
· * External email address: Use this box to type the outside email account of the contact. This box is required. Email sent to this contact is forwarded
to this email address.
· Organizational unit: You can select an organizational unit (OU) other than the default, which is the recipient scope. If the recipient scope is
set to the forest, the default value is set to the Users container in the domain that contains the computer on which the EAC is running. If the recipient scope is set to a specific domain, the Users container in that domain is selected by default. If the recipient
scope is set to a specific OU, that OU is selected by default.
To select a different OU, click Browse. The dialog box displays all OUs in the forest that are within the specified scope. Select the OU you want, and then click
OK.
Note: The Organizational unit box is only available in Exchange Server. It isn't available in Exchange Online.
4. When you're finished, click
Save.
B. Open your O365 group from Outlook Web App : Click on Add members and Enter the specific mail contact's email id and save the changes.
For Create a mail contact, you can refer this article: https://docs.microsoft.com/en-us/exchange/recipients-in-exchange-online/manage-mail-contacts#create-a-mail-contact
Regards,
Ankita Vaidya