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With the formula =VLOOKUP(RAND(),A3:B6,2), if RAND() generates a value less than the value in A3, VLOOKUP will return #N/A.
So the value in A3 should be zero or negative in order to ensure that VLOOKUP always work.
Moreover, it should go without saying that the values in A3:A6 should be numeric and in ascending order.
However, other than the requirement above regarding A3, the values in A4:A6 can be anything.
In particular, they do not need to include 1. In fact, they do not even need to be less than 1 -- although arguably, the VLOOKUP expression seems pointless if they are greater than 1.