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Add One URL to Intranet Zone and Another URL to a Trusted Site Zone Through GPO-ADM

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Please note: If you want to manage Trusted/Intranet site through GPO, end users will be not able to add their sites.The below ADM was tested and there's a link for a VB Script. You can use one of them.

;;;;Add one URL to Intranet Zone and Another Url To  trusted Site Zone through GPO-ADM
 ;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;
 CLASS USER                     ;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;
 ;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;
 CATEGORY !!INTRANET_TRUSTED
  
    ;;--------
     ;; Feature: Intranet trusted
     ;;--------
      
    POLICY "Domaincontosohttp"
  KEYNAME "Software\Microsoft\Windows\CurrentVersion\Internet Settings\ZoneMap\Domains\contoso.com"
     EXPLAIN !!ExplainText_ConfigurationMode
         VALUENAME "http"
         VALUEON   NUMERIC  2
         VALUEOFF  NUMERIC  0
     END POLICY
  
    POLICY "Domaincontosohttps"
  KEYNAME "Software\Microsoft\Windows\CurrentVersion\Internet Settings\ZoneMap\Domains\contoso.com"
     EXPLAIN !!ExplainText_ConfigurationMode
         VALUENAME "https"
         VALUEON   NUMERIC  2
         VALUEOFF  NUMERIC  0
 END POLICY
  
POLICY "contosoEschttp"
  KEYNAME "Software\Microsoft\Windows\CurrentVersion\Internet Settings\ZoneMap\EscDomains\contoso.com"
     EXPLAIN !!ExplainText_ConfigurationMode
         VALUENAME "http"
         VALUEON   NUMERIC  2
         VALUEOFF  NUMERIC  0
     END POLICY
      
POLICY "contosoEschttps"
  KEYNAME "Software\Microsoft\Windows\CurrentVersion\Internet Settings\ZoneMap\EscDomains\contoso.com"
     EXPLAIN !!ExplainText_ConfigurationMode
         VALUENAME "https"
         VALUEON   NUMERIC  2
         VALUEOFF  NUMERIC  0
 END POLICY
  
END CATEGORY ; INTRANET_TRUSTED
  
;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;;
  
[strings]
 INTRANET_TRUSTED="Trusted sites for IE"
  
ExplainText_ConfigurationMode="Enable or disable listed servers"

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If you require the VB Script, find the below link.
http://social.technet.microsoft.com/wiki/contents/articles/add-one-url-to-intranet-zone-and-another-url-to-a-trusted-site-zone-through-gpo.aspx