@EnterpriseArchitect, Thanks for posting in Q&A. Based on my experience, if the records are still in Azure AD, we can remove these Hybrid Azure AD joined device records in Azure AD portal.
Meanwhile, if you want to just do Hybrid Azure AD join for some devices, you can create an OU to put the users and devices you want, configure the customize synchronization options in Azure AD connect to only sync the users and devices in your specific OU.
Hope the above information can help.
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