You have an option in the Folder Options window, under the "General" tab, in the "Privacy" section to reset quick access.
How to manuelly remove a quick access item when Unpin doesn't work.
Brandon Kline
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So I uninstalled Onedrive, and in registry changed the Documents, Desktop, Pictures, etc stuff over to local, but when I go to unpin one drive's versions of stuff in quick access and I am able to remove everything EXCEPT pictures. I click unpin from the right-click menu and nothing happens. Is there any file I can edit to manually remove it?
EDIT: Nevermind. deleting / moving the pictures folder from the onedrive folder removed it. Weird don't know why it wouldn't let me unpin it. Oh well.