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Hi Andy,
Does the problem occur to all devices which you sync the OneDrive for Business library to? If so, you may first check whether there are unsupported file types or formats in cloud that can’t be synced to the local client:
https://support.microsoft.com/en-us/kb/2933738
After making sure that all files are under the sync limits, please stop syncing the folder and navigate to the following folders to remove all files:
C:\Users%USERPROFILE%\AppData\Local\Microsoft\Office\16.0\OfficeFileCacheC:\Users%USERPROFILE%\AppData\Local\Microsoft\Office\Spw
Let us know if there is any improvement re-syncing the affected library.
Regards,
Jerry