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Hi Hilary,
You can try the fix it tool in this article to remove the cache of OneDrive for Business, and then check the outcome.
Note:Please back up those important files. It may take some time finish the process.
If the issue persists, I’d like to confirm the following things for further investigation:
1.Open one of the Office applications>File>Account>capture a screenshot of Product Information.
2.Check the version of OneDrive for Business. Please also follow the steps in the article below to check the version of Microsoft Office Document Cache (MSOSYNC.EXE)
How to determine the version of OneDrive for Business Sync client
3.The screenshot of the error message. Moreover, is there a yellow mark on the OneDrive for Business icon in the task bar? When you right-click the icon, can you click View sync problems? If yes, please also capture a screenshot of the pop-up.
4.If it’s convenient, can you change to another computer and sync your OneDrive for Business library to see the result. Meanwhile, does OneDrive for Business work well before? When do you encounter this issue, after updating the Office or Windows?
Thanks for your time.
Tim